Really hard question...I don't know if it's easy to separate actors from their vehicles...good movies make good actors while good actors don't necessarily make good movies...I'll list my personal favorites rather than claim they are the "best":
Male:
1) Anthony Hopkins
2) David Boreanz
3) Richard Burton
4) Roy Dupuis
Female:
1) Sarah Michelle Gellar
2) Alyson Hannigan
3) Merryl Streep
4) Juliette Lewis
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